Experimental and computational insight into the properties of the lattice-mismatched structures: Monolayers of h-BN and graphene on Ir(111)

Author(s)
Dmitry Usachov, Alexander V. Fedorov, Oleg Vilkov, Vera K. Adamchuk, Lada V. Yashina, L. V. Bondarenko, Alexander A. Saranin, Alexander Grüneis, D.V. Vyalikh
Abstract

We report a comparative study of the synthesis and the structural and electronic properties of hexagonal boron nitride (h-BN) and graphene layers grown on the Ir(111) surface. By performing photoemission (PE) experiments time-dependently and supplementing them by low-energy electron diffraction (LEED) data, we demonstrate the differences and similarities of their formation, and we show the temperature regimes which allow these materials to be created with high crystalline quality. It has been demonstrated that synthesis at low temperatures leads to the formation of disordered domains of h-BN as well as graphene flakes on the metallic surface. The LEED patterns of such samples reveal a complex structure which indeed can be easily interpreted by using the model presented here. The angle-resolved PE study of h-BN/Ir(111) demonstrates the presence of replicated electronic states, which are quite similar to those detected and widely discussed for the graphene/Ir(111) system. On the basis of these results and the corresponding model calculations, we argue that the appearance of these replicated bands is mainly caused by the geometrical corrugation of the system.

Organisation(s)
Electronic Properties of Materials
External organisation(s)
Saint Petersburg State University, Anuchin Research Institute and Museum of Anthropology, Far Eastern Federal University, Technische Universität Dresden
Journal
Physical Review B
Volume
86
No. of pages
9
ISSN
1098-0121
DOI
https://doi.org/10.1103/PhysRevB.86.155151
Publication date
2012
Peer reviewed
Yes
Austrian Fields of Science 2012
103015 Condensed matter
Portal url
https://ucrisportal.univie.ac.at/en/publications/experimental-and-computational-insight-into-the-properties-of-the-latticemismatched-structures-monolayers-of-hbn-and-graphene-on-ir111(abf5d0d3-2186-4c0d-99ce-242bbfff68f0).html